Open Access

The Duffing equation containing a cubic nonlinearity is probably the most popular example of a nonlinear oscillator. For its harmonically excited, slightly damped, and softening version, stationary large amplitude solutions at subcritical excitation frequencies are obtained when standard semi-analytical methods like Harmonic Balance or Perturbation Analysis are applied. These solutions have the shape of a nose in the amplitude-frequency diagram. In prior work, it has been observed that these solutions may contain large errors and that high ansatz orders may be necessary when applying the Harmonic Balance or other semi-analytical methods to make them converge. Some of these solutions are observed to be asymptotically stable, while in most cases, they are unstable. The current paper aims to give a descriptive explanation for this behavior of the nose solutions, which is mainly related to the exact solution of the free undamped vibrations. Based on this, approximations of the nose solutions are calculated with a procedure combining properties of Perturbation Analysis and Harmonic Balance. Therein, the exact solution of the free undamped vibrations is taken as the zeroth approximation, while higher-order solution parts are calculated by balancing the harmonics, and the phase shift of the zeroth approximation is calculated by a residuum minimization. This method just requires the solution of a system of linear algebraic equations, while systems of nonlinear algebraic equations have to be solved in the case of directly applying Harmonic Balance.

Many borate crystals feature nonlinear optical properties that allow for efficient frequency conversion of common lasers down into the ultraviolet spectrum. Twinning may degrade crystal quality and affect nonlinear optical properties, in particular if crystals are composed of twin domains with opposing polarities. Here, we use measurements of optical activity to demonstrate the existence of inversion twins within single crystals of YAl3(BO3)4 (YAB) and K2Al2B2O7 (KABO). We determine the optical rotatory dispersion of YAB and KABO throughout the visible spectrum using a spectrophotometer with rotatable polarizers. Space-resolved measurements of the optical rotation can be related to the twin structure and give estimates on the extent of twinning. The reported dispersion relations for the rotatory power of YAB and KABO may be used to assess crystal quality and to select twin-free specimens.